Volume 7, Issue 1
Theoretical Exploration of the Interference Minimum in Molecular High-Order Harmonic Generation

Liqing Li, Yuanyuan Xu & Xiangyang Miao

J. At. Mol. Sci., 7 (2016), pp. 1-10.

Published online: 2016-07

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  • Abstract

The interference minimum in the molecular high-order harmonic generation is studied by numerically solving the non-Born-Oppenheimer approximation time-dependent Schrödinger equation. The results show that two kinds of interference minima appear in the high-order harmonic spectrum when the hydrogen molecular ion is exposed to the laser pulse. Furthermore, by adjusting wavelength of the laser as well as initial condition of nucleus, it is found that two kinds of interference minima are ascribed to the molecular structure and the electronic dynamics behavior induced by the laser field, respectively. Besides, the time-frequency distributions and the electron wave packet distributions are calculated to better understand the mechanism of the minimum.

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COPYRIGHT: © Global Science Press

  • Email address

sxxymiao@126.com (Xiangyang Miao)

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@Article{JAMS-7-1, author = {Li , LiqingXu , Yuanyuan and Miao , Xiangyang}, title = {Theoretical Exploration of the Interference Minimum in Molecular High-Order Harmonic Generation}, journal = {Journal of Atomic and Molecular Sciences}, year = {2016}, volume = {7}, number = {1}, pages = {1--10}, abstract = {

The interference minimum in the molecular high-order harmonic generation is studied by numerically solving the non-Born-Oppenheimer approximation time-dependent Schrödinger equation. The results show that two kinds of interference minima appear in the high-order harmonic spectrum when the hydrogen molecular ion is exposed to the laser pulse. Furthermore, by adjusting wavelength of the laser as well as initial condition of nucleus, it is found that two kinds of interference minima are ascribed to the molecular structure and the electronic dynamics behavior induced by the laser field, respectively. Besides, the time-frequency distributions and the electron wave packet distributions are calculated to better understand the mechanism of the minimum.

}, issn = {2079-7346}, doi = {https://doi.org/10.4208/jams.080815.091015a}, url = {http://global-sci.org/intro/article_detail/jams/8099.html} }
TY - JOUR T1 - Theoretical Exploration of the Interference Minimum in Molecular High-Order Harmonic Generation AU - Li , Liqing AU - Xu , Yuanyuan AU - Miao , Xiangyang JO - Journal of Atomic and Molecular Sciences VL - 1 SP - 1 EP - 10 PY - 2016 DA - 2016/07 SN - 7 DO - http://doi.org/10.4208/jams.080815.091015a UR - https://global-sci.org/intro/article_detail/jams/8099.html KW - High-order harmonic generation, Interference minimum, Non-Born-Oppenheimer approximation. AB -

The interference minimum in the molecular high-order harmonic generation is studied by numerically solving the non-Born-Oppenheimer approximation time-dependent Schrödinger equation. The results show that two kinds of interference minima appear in the high-order harmonic spectrum when the hydrogen molecular ion is exposed to the laser pulse. Furthermore, by adjusting wavelength of the laser as well as initial condition of nucleus, it is found that two kinds of interference minima are ascribed to the molecular structure and the electronic dynamics behavior induced by the laser field, respectively. Besides, the time-frequency distributions and the electron wave packet distributions are calculated to better understand the mechanism of the minimum.

Li , LiqingXu , Yuanyuan and Miao , Xiangyang. (2016). Theoretical Exploration of the Interference Minimum in Molecular High-Order Harmonic Generation. Journal of Atomic and Molecular Sciences. 7 (1). 1-10. doi:10.4208/jams.080815.091015a
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