TY - JOUR T1 - Photon Statistical Properties Emitted from Single Molecule Derived from Generating Function Method AU - Han , Baiping JO - Journal of Atomic and Molecular Sciences VL - 4 SP - 191 EP - 199 PY - 2016 DA - 2016/07 SN - 7 DO - http://doi.org/10.4208/jams.052516.081516a UR - https://global-sci.org/intro/article_detail/jams/8158.html KW - Two-Level System, Generating Function, Photon Counting Statistics. AB -
In this paper, we summarize the photon emission statistical properties of single molecule system, using the recently developed generating function method. Through the introduce of one or double “auxiliary” variables, we can investigate the first moment and second moment of photon emission statistics driven by different external fields, such as the line shapes and Mandel's Q parameters, the photon emission probabilities, the probability distribution of time between successive emission, the waiting time and the waiting time distribution, the cross correlation, the joint probabilities, etc. Among, the first moment of photon statistics and the experimental results of optical amplification are in good agreement.